Popsugar Entertainment The Vampire Diaries Caroline and Stefan GIFs From The Vampire Diaries The Romantic Evolution of Stefan and Caroline's Relationship March 9, 2017 by Sundi Rose View On One Page Photo 4 of 24 ADVERTISEMENT () Start Slideshow Share This Link Copy ← Use Arrow Keys → 4 Longing Looks These two take pining to a whole new level. Even when they are together, the dreamy longing is pretty thick. Previous Next Start Slideshow The Vampire DiariesTV